This dataset provides information on greenhouse gases and human-produced air pollution, including atmospheric concentrations of carbon dioxide (CO2), methane (CH4), tropospheric ozone (O3), and black carbon (BC) aerosols, collected during airborne campaigns conducted by NASA's Atmospheric Tomography (ATom) mission. This dataset includes merged data from all instruments plus additional data such as numbered profiles and distance flown. Merged data products have been created for seven different aggregation intervals (1 second, 10 seconds, and 5 instrument-specific intervals). In the case of data obtained over longer time intervals (e.g., flask data), the merge files provide (weighted) averages to match the sampling intervals. This comprehensive dataset will be used to improve the representation of chemically reactive gases and short-lived climate forcers in global models of atmospheric chemistry and climate.

This dataset provides Modeling Data Stream (MDS) and Reactivity Data Stream (RDS) products for each of the four ATom campaigns conducted from 2016 to 2018. MDS files contain the atmospheric constituents needed to model the RDS of the air parcels along ATom flight paths. The MDS is a continuous data stream (every 10 seconds) of the atmospheric content of these key chemical species derived from the in-situ measurements collected along ATom flight paths (as reported in the comprehensive related dataset ATom: Merged Atmospheric Chemistry, Trace Gases, and Aerosols). Values for chemical species measured by multiple instruments were selected from the instrument with better coverage and/or greater precision. Missing values were filled using interpolation for short gaps. For long gaps owing to instrument failure, values were estimated using multiple linear regressions from comparable parallel flights from other ATom campaigns. All species were flagged for instrument source and values were flagged for gap-filling status. In combination, MDS and RDS provide, in essence, a photochemical climatology for each air parcel along ATom flight paths containing the reactive species that control the loss of methane and the production and loss of ozone.

This dataset consists of (a) selected aerosol and gas-phase observations made on all four deployments of NASA Atmospheric Tomography Mission (ATom), (b) thermodynamic properties related to aerosol formation derived from these measurements, (c) 48-h back trajectories for ATom-4 observations, and (d) output from the Model of Aerosols and Ions in the Atmosphere (MAIA). ATom observations, thermodynamics, and back trajectories were inputs for MAIA model runs. MAIA runs focused on data from ATom-4 deployment, and output includes aerosol formation rates, and ultrafine particle size distributions and number concentrations in the lowermost stratosphere (LMS). ATom 1-4 deployments included all four seasons from 2016 to 2018. This investigation sought to understand how new particle formation (NPF) can occur in the LMS, factors influencing the amount of NPF, and other potential sources of ultrafine aerosols in this region of the atmosphere. The data are provided in comma-separated value (CSV) format.

This dataset contains comprehensive measurements of aerosol microphysical, chemical, and optical properties derived for both dry and ambient conditions from in situ measurements made during the four ATom campaigns. The dataset includes composition-resolved size distributions the integrated mass of sulfate, organics, nitrate, sea salt, dust, black carbon, and other compounds in coarse and fine fractions; extinction and absorption coefficients from each species at both dry and ambient conditions; asymmetry parameters; Angstrom exponents; and fitted lognormal functions to describe the size distribution. Optical parameters are calculated for 10 wavelengths from the near UV to the near IR, and size distributions range from 3 nm to 50 um in diameter. One file contains these data at 1-minute time intervals. Another file contains a subset of these data averaged into 1-km vertical bins for each vertical profile the aircraft made, as well as composition-resolved integrated aerosol optical depth derived from each profile. The concentration of cloud condensation nuclei is calculated for 5 supersaturations.

This dataset consists of (a) selected aerosol and gas-phase observations made on all four deployments of NASA Atmospheric Tomography Mission (ATom), (b) thermodynamic properties related to aerosol formation derived from these measurements, (c) 48-h back trajectories for ATom-4 observations, and (d) output from the Model of Aerosols and Ions in the Atmosphere (MAIA). ATom observations, thermodynamics, and back trajectories were inputs for MAIA model runs. MAIA runs focused on data from ATom-4 deployment, and output includes aerosol formation rates, and ultrafine particle size distributions and number concentrations in the lowermost stratosphere (LMS). ATom 1-4 deployments included all four seasons from 2016 to 2018. This investigation sought to understand how new particle formation (NPF) can occur in the LMS, factors influencing the amount of NPF, and other potential sources of ultrafine aerosols in this region of the atmosphere. The data are provided in comma-separated value (CSV) format.

This dataset provides (1) the results of in situ aerosol particle property measurements collected over remote tropical areas of both Pacific and Atlantic Oceans during the NASA airborne Atmospheric Tomography (ATom) campaigns for ATom-1 and ATom-2 and (2) modeled outputs of comparable aerosol properties, atmospheric chemistry and meteorology at 70 m resolution from four chemical-transport models matched to the location and time of the aircraft measurements.

Soluble acidic gases and aerosols (SAGA) were collected with two related installations; a mist chamber/ion chromatography (MC/IC) system and a paired bulk aerosol system. The MC/IC system measures in situ atmospheric distributions of nitric acid (plus < 1 um NO3 aerosol) and fine (< 1 um) aerosol sulfate at an approximately 80-second interval. The paired bulk aerosol system collects particulates onto filters for subsequent analysis. Collected filters were first extracted with water to obtain the water-soluble (WS) constituents and then extracted again using methanol to collect the methanol soluble (MS) fraction. The light absorption of filtered extracts was measured from 300 to 700 nm. Ion chromatography on aqueous extracts of the bulk aerosol samples collected on Teflon filters were used to quantify soluble ions (Cl-, Br-, NO3-, SO42-, C2O42-, Na+, NH4+, K+, Ca+, and Mg+). The SAGA system is provided by the University of New Hampshire (UNH).

This dataset provides information on greenhouse gases and human-produced air pollution, including atmospheric concentrations of carbon dioxide (CO2), methane (CH4), tropospheric ozone (O3), and black carbon (BC) aerosols, collected during airborne campaigns conducted by NASA's Atmospheric Tomography (ATom) mission. This dataset includes merged data from all instruments plus additional data such as numbered profiles and distance flown. Merged data have been created for seven different sampling intervals. In the case of data obtained over longer time intervals (e.g. flask data), the merge files provide (weighted) averages to match the sampling intervals. ATom deploys an extensive gas and aerosol payload on the NASA DC-8 aircraft for a systematic, global-scale sampling of the atmosphere, profiling continuously from 0.2 to 12 km altitude. Flights occurred in each of 4 seasons from 2016 to 2018. Flights originate from the Armstrong Flight Research Center in Palmdale, California, fly north to the western Arctic, south to the South Pacific, east to the Atlantic, north to Greenland, and return to California across central North America. ATom establishes a single, contiguous, global-scale dataset. This comprehensive dataset will be used to improve the representation of chemically reactive gases and short-lived climate forcers in global models of atmospheric chemistry and climate. Profiles of the reactive gases will also provide critical information for the validation of satellite data, particularly in remote areas where in situ data is lacking. Complete aircraft flight information including, but not limited to, latitude, longitude, and altitude are also provided. This data release provides results from all instruments on all four ATom flight campaigns.

This dataset, collected with the Unmanned Aircraft Systems (UAS) Chromatograph for Atmospheric Trace Species (UCATS), provides atmospheric concentrations of nitrous oxide (N2O), sulfur hexafluoride (SF6), methane (CH4), hydrogen (H2), carbon monoxide (CO), water vapor (H2O), and ozone (O3). The UCATS system is three different instruments in one enclosure: a two-channel chromatograph with electron capture detectors (one measures N2O and SF6, the other measures CH4, H2 and CO), a tunable diode laser instrument for H2O, and a dual-beam O3 photometer.

This dataset provides calculated age of air (AoA) and the argon/nitrogen (Ar/N2) ratio (per meg) from stratospheric flask samples and simultaneous high-frequency measurements of nitrous oxide (N2O), carbon dioxide (CO2), ozone (O3), methane (CH4), and carbon monoxide (CO) compiled from three airborne projects. The trace gases were used to identify 235 flask samples with stratospheric influence collected by the Medusa Whole Air Sampler and to calculate AoA using a new N2O-AoA relationship developed using a Markov Chain Monte Carlo algorithm. The data span a wide range of latitudes poleward of 40 degrees in both the Northern and Southern Hemispheres and cover the period 2009-01-10 to 2018-05-21.