Data for "Quantum state tracking and control of a single molecular ion in a thermal environment''
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Supplementary data for the article "Quantum state tracking and control of a single molecular ion in a thermal environment" by Yu Liu, Julian Schmidt, Zhimin Liu, David R. Leibrandt, Dietrich Leibfried, Chin-wen Chou, submitted to Science in 2024. The manuscript describes a quantum state-specific investigation of the molecular state evolution of a single CaH+ ion in a thermal environment. The molecular state can be tracked in real time with single quantum-state resolution and the thermal radiation-induced transitions can be reversed with coherent molecular state manipulation according to the outcomes of state measurements. Results on the transition rates are used to infer the properties of the thermal environment. The data may be used to reproduce the plots shown in the figures.
Data associated with "Two-dimensional imaging of electromagnetic fields via light sheet fluorescence imaging with Rydberg atoms"
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Data associated with the publication: "Two-dimensional imaging of electromagnetic fields via light sheet fluorescence imaging with Rydberg atoms"Abstract:The ability to image electromagnetic fields holds key scientific and industrial applications, including electromagnetic compatibility, diagnostics of high-frequency devices, and experimental scientific work involving field interactions. Generally electric and magnetic field measurements require conductive elements which significantly perturb the field. However, electromagnetic fields can be measured non-perturbatively via the shift they induce on Rydberg states of alkali atoms in atomic vapor, which are highly sensitive to electric fields. Previous field measurements using Rydberg atoms utilized electromagnetically induced transparency to read out the shift on the states induced by the fields, but did not provide spatial resolution. In this work, we demonstrate that electromagnetically induced transparency can be spatially resolved by imaging the fluorescence of the probe. We demonstrate that this can be used to image $\sim$V/cm scale electric fields in the MHz-GHz range and $\sim$mT scale static magnetic fields, with minimal perturbation to the fields. We also demonstrate the ability to image $\sim$ V/m scale fields for resonant microwave radiation, although standing waves generated by the vapor cell walls obscure external field structure in this regime. We perform this field imaging with a spatial resolution of order 160 $\mu$m.This dataset contains the data associated with Figure 1 c,f,g, and h, Figure 2, Figure 3 b,d,f, and h, Figure 4 c,d, and e, Figure 5 b, c, and e, Figure 6, and the Supplemental Material's Figure 1.
Data for "Frequency-comb spectroscopy on pure quantum states of a single molecular ion"
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These data files contain the data for the measured transition frequencies shown in Table I and the traces in Figure 3 of the publication "Frequency-comb spectroscopy on pure quantum states of a single molecular ion," accessible at https://arxiv.org/abs/1911.12808. In this publication we use generally applicable quantum-logic techniques to prepare a trapped molecular ion in a single quantum state, drive terahertz rotational transitions with an optical frequency comb, and read out the molecular state non-destructively, leaving the molecule ready for further manipulation. One file contains data For Table 1. In the measurement of rotational transition frequencies, the intensities of the comb beams are varied to characterize the effect of AC Stark shift, while the intensity ratio between the sigma and pi polarized beams are kept at close to 2. The average intensity of the sigma-polarized comb beam is quantified by measuring the resultant Stark shift, fSS_sigma, on the 729 nm transition of the Ca+ ion, with the Ca+ ion where the CaH+ ion would be during rotational spectroscopy experiments. The other file contains data for Figure 3, (a) Spectra for the J = 4 to 2 transition: 40CaH+ is prepared in J = 2, followed by a pulse train from the comb Raman beams probing the J = 2 to J = 4 transition. After the probe pulse train, projective measurements of both initial and final states are performed and the state occupation probability is determined. The probe time is ~1.6 ms. The frequency shows the offset of the Raman difference frequency from the resonant value. (b) Rabi flopping on the J = 4 to J = 2 transition: Starting in J = 4, with the comb Raman pulse detuning set to resonance, the state of the 40CaH+ ion is driven coherently to J = 2 by a pulse train of variable duration from the comb Raman beams. The center wavelength of the frequency comb was ~800 nm for these spectra and Rabi flopping traces. The error bars stand for ±1 standard deviation.
Data for the article " Pseudo-resonant Detection of `Low Frequency' VHF Electric Fields via Rabi Matching with Autler-Townes Splitting in Rydberg Atoms"
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This dataset represents absorption/transmission spectra of resonant probe light power through a Rydberg atom vapor, subject to a simultaneous dressing field and a 'low frequency' field. Data is taken as an oscilloscope average of 5 photodiode voltage traces, with frequency offsets given by a simultaneous reference cell (not included). Some data are given as 2-D arrays, with axes of laser detuning across a waterfall of field strength. Some data represents theory eigen-energies of the system, for comparison. This paper will be submitted to Physical Review Letters.
Data associated with "Zeeman-resolved Autler-Townes splitting in Rydberg atoms with a tunable RF resonance and a single transition dipole moment"
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Data associated with the publication: "Zeeman-resolved Autler-Townes splitting in Rydberg atoms with a tunable RF resonance and a single transition dipole moment"Applying a magnetic field as a method for tuning the frequency of Autler-Townes splitting for Rydberg electrometry has recently been demonstrated. In the corresponding paper, we provide a theoretical understanding of EIT signals in the presence of a large magnetic field, as well as demonstrate some advantages of this technique over traditional Autler-Townes based electrometry. We show that a strong magnetic field provides a well-defined quantization axis regardless of the optical field polarizations, we demonstrate that by separating the $m_J$ levels of the Rydberg state we can perform an Autler-Townes splitting with a single participating dipole moment, and we demonstrate recovery of signal strength by populating a single $m_J$ level using circularly polarized light.Included in this dataset is the data associated with every plot in the paper, separated by figure number, including:FIgure 2: Measured EIT signals in the presence of a strong(1.85(1) mT) magnetic field either aligned with or orthogonalto the polarization axis. Figure 3: Theoretical EIT signals for Cs in the presence ofa 1.85(1) mT magnetic field for light polarizations alignedto or orthogonal to the magnetic field.Figure 4: Measured Autler-Townes splittings in individual mJlevels via the 58D5/2(mJ = ±5/2) ? 59P3/2(mJ = ±3/2)transitions of Cs in the presence of 2.78(1) mT.Figure 5: Measured Autler-Townes splittings on the Cs58D5/2 ? 59P3/2 transition with and without mJ selectivityfor various RF fields up to 3.08 V/m. Figure 6: EIT in the presence of a large magnetic field using circularly polarized light.EIT signals correspond to voltage traces (collected on an oscilloscope) of a balanced photodiode as laser frequencies are scanned. The x axis is converted from a time series of each voltage to a frequency using a reference cell. The scaling is determined by measuring the difference between the EIT peaks corresponding to the D5/2 and D3/2 Rydberg states, and the zero is generally taken to be the location of the D5/2 EIT peak.
Phase-shift Data for Fully Quantum Calculations of Thermophysical Properties for Noble Gases
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This data deposit contains JSON files of phase-shift data and related quantities for pair interactions using state-of-the-art pair potentials for helium (isotopes of mass 3 and 4 and their cross interaction), neon (all six interactions among isotopes with masses 20, 21, and 22), and argon (the dominant isotope of mass 40). A Python program is supplied to compute the second virial coefficient B(T), its first two temperature derivatives, and the second acoustic virial coefficient for any of these pair interactions at temperatures up to 1500 K. The lower temperature limit is 0.01 K for helium, 1 K for neon, and 10 K for argon. Another program is supplied to calculate these quantities for neon of natural isotopic composition.This work is described in a paper: G. Garberoglio and A.H. Harvey, "Avoiding Interpolation Errors for Computed Second Virial Coefficients of Noble Gases", Metrologia, in preparation (2025).The code and data files are also maintained at this Github site:https://github.com/gioGarbe/TAPPS