Measurements taken during the Aerosol Characterization Experiment (ACE) off the coast of Spain, Portugal, and Northern Africa in the Atlantic Ocean.

Measurements taken during the Aerosol Characterization Experiment (ACE) off the coast of Asia in the East China Sea, Sea of Japan, and Pacific Ocean.

Measurements made as a part of the Aerosol Characterization Experiment (ACE) for the in-land Chesapeake Bay region between 2002 and 2003.

Measurements made as a part of the Aerosol Characterization Experiment (ACE) for the in-land Chesapeake Bay region between 2002 and 2003.

This dataset provides observations collected during eleven airborne campaigns from 2006–2017 and associated input and output from nine widely used chemical transport models (CTMs). The airborne campaigns include ARCTAS-A, ARCTAS-B, ATom-1 and ATom-2, CalNex, DC3, INTEX-B, KORUS-AQ, MILAGRO, SEAC4RS, and WINTER, and they sampled mainly tropospheric air over the conterminous U.S. and the state of Alaska, Mexico, Canada, Greenland, and South Korea and remote areas over the Arctic, Pacific, Southern, and Atlantic Oceans. The CTMs are the AM4.1, CCSM4, GEOS-5, GEOS-Chem TOMAS, GEOS-Chem v10, GEOS-Chem v12, GISS-MATRIX, GISS-ModelE, and TM4-ECPL-F, and the output includes sulfate, nitrate, temperature, specific humidity, mixing ratio of ammonium, the volume mixing ratio of nitric acid, surface pressure, gas-phase ammonia, gas-phase nitric acid, pressure, total ammonium, etc. The observations were collected in-situ from a variety of instruments, including the Aerosol Microphysical Properties (AMP), HR Aerodyne Aerosol Mass Spectrometer (AMS), CIT Chemical Ionization Mass Spectrometer (CIMS), diode laser hygrometer (DLH), a mist chamber/ion chromatography system (MC/IC), Particle Analysis by Laser Mass Spectrometer (PALMS), Single Particle Soot Photometer (SP2), and UCI Whole Air Sampler (WAS). In-situ data also include latitude, longitude, and pressure. These observations were used to investigate how aerosol pH and ammonium balance change from polluted to remote regions, such as over oceans, and were compared to predictions from the CTMs.

This dataset provides (1) the results of in situ aerosol particle property measurements collected over remote tropical areas of both Pacific and Atlantic Oceans during the NASA airborne Atmospheric Tomography (ATom) campaigns for ATom-1 and ATom-2 and (2) modeled outputs of comparable aerosol properties, atmospheric chemistry and meteorology at 70 m resolution from four chemical-transport models matched to the location and time of the aircraft measurements.

This dataset provides (1) the results of in situ aerosol particle property measurements collected over remote tropical areas of both Pacific and Atlantic Oceans during the NASA airborne Atmospheric Tomography (ATom) campaigns for ATom-1 and ATom-2 and (2) modeled outputs of comparable aerosol properties, atmospheric chemistry and meteorology at 70 m resolution from four chemical-transport models matched to the location and time of the aircraft measurements.

Measurements made near Spain and Portugal under the AOPEX program.

Aerosol measurements began at the NOAA Earth System Research Laboratory (ESRL) Global Monitoring Division (GMD) baseline observatories in the mid-1970's with the purpose of detecting a response, or lack of response, of atmospheric aerosols to changing conditions on a global scale. In 1992 ESRL/GMD expanded its aerosol research program to include regional aerosol monitoring stations due to anthropogenic aerosols creating a significant perturbation in the Earth's radiative balance on regional scales. The goals of this regional-scale monitoring program are to characterize means, variability, and trends of climate-forcing properties of different types of aerosols, and the factors that control them. In situ measurements of aerosol optical properties (including light absorption, total scattering, hemispheric backscattering, and total aerosol number concentration) are made at monitoring sites at hourly time resolution. The basic aerosol measurement system consists of a nephelometer (measures aerosol light scattering), absorption photometer (measures light absorption), and a condensation nuclei counter (measures particle number concentration). Data from the aerosol monitoring stations are updated several times a day. Following collection of the raw data at the station, the data are inspected through automatic and manual contamination screenings to eliminate contamination from local pollution sources. Automatic screenings use measured wind speed, direction, and/or total particle number concentration to flag contaminated data. Manual screening is more subjective, relying on the station scientist to evaluate the data in the context of automated contamination flags and their knowledge of the site. Data applications indicate the importance of continuing to provide long-term aerosol in-situ measurements for use in analysis of trends and climatologies, evaluation of model simulations of aerosol climatologies, and behavior and validation of remote sensing retrievals of aerosol optical properties. GMD's measurements also provide ground-truth for satellite measurements and global models, as well as key aerosol parameters for global-scale models. Through the Big Earth Data Initiative (BEDI), ESRL/GMD has taken their data collection and converted files into NetCDF-4, a self-describing format.

This dataset provides observations collected during eleven airborne campaigns from 2006–2017 and associated input and output from nine widely used chemical transport models (CTMs). The airborne campaigns include ARCTAS-A, ARCTAS-B, ATom-1 and ATom-2, CalNex, DC3, INTEX-B, KORUS-AQ, MILAGRO, SEAC4RS, and WINTER, and they sampled mainly tropospheric air over the conterminous U.S. and the state of Alaska, Mexico, Canada, Greenland, and South Korea and remote areas over the Arctic, Pacific, Southern, and Atlantic Oceans. The CTMs are the AM4.1, CCSM4, GEOS-5, GEOS-Chem TOMAS, GEOS-Chem v10, GEOS-Chem v12, GISS-MATRIX, GISS-ModelE, and TM4-ECPL-F, and the output includes sulfate, nitrate, temperature, specific humidity, mixing ratio of ammonium, the volume mixing ratio of nitric acid, surface pressure, gas-phase ammonia, gas-phase nitric acid, pressure, total ammonium, etc. The observations were collected in-situ from a variety of instruments, including the Aerosol Microphysical Properties (AMP), HR Aerodyne Aerosol Mass Spectrometer (AMS), CIT Chemical Ionization Mass Spectrometer (CIMS), diode laser hygrometer (DLH), a mist chamber/ion chromatography system (MC/IC), Particle Analysis by Laser Mass Spectrometer (PALMS), Single Particle Soot Photometer (SP2), and UCI Whole Air Sampler (WAS). In-situ data also include latitude, longitude, and pressure. These observations were used to investigate how aerosol pH and ammonium balance change from polluted to remote regions, such as over oceans, and were compared to predictions from the CTMs.